The First Nuclear Era: The Life and Times of Nuclear Fixer by Alvin M. Weinberg (Hardcover, 1997)

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This book is his autobiography and it's peppered with first-hand accounts of major historical events. He writes about the events of December 2, 1942, when Fermi set into motion the first chain reaction in a uranium pile and goes on to describe what happened during the "First Nuclear Era" a period he admits that has now largely run its course.